Semiconductors Research

With the emergence of two-dimensional semiconductor materials, it became evident that they host highly stable few-body bound states, characterized by their strong interaction with light. This has led to a wide range of innovative technological applications that leverage the unique properties of these quasiparticles. One of the key applications is found in excitons, which are the bound states of an electron and a hole. Excitons have been instrumental in advancing technologies such as photodetectors, solar cells, LEDs, quantum emitters, nonlinear optics, and chirality logic gates. However, our project aims to go beyond the realm of excitons to explore more complex few-body states. These include trions (charged excitons or the bound state of three electrons and holes), biexcitons (the bound state of two electrons and two holes), and quintons (charged biexcitons or the bound state of five electrons and holes). Trions, in particular, have shown immense potential in optical experiments involving doped samples. These samples can be created through electrostatic gating, subtract charge transfer processes, or chemical methods. An increase in doping levels leads to a notable shift in the exciton's oscillator strength towards the trion, leading to a trion-Fermi polaron transition. Biexcitons, representing four-body neutral bound states in semiconductors, are crucial for understanding the nonlinear optical properties of these materials. Moreover, biexcitons are key players in quantum technologies, especially as mediators for parametric-down conversion in nonlinear anisotropic crystals. Our focus on these confined few-body complexes is driven by their high quantum yield, positioning them as invaluable single-photon sources for various quantum technologies like quantum communication, quantum sensing, and quantum computation.

This collaborative initiative involves researchers from Central State University and Brazilian collaborators from Aeronautics Institute of Technology and the Federal University of Ceará. This collaboration aims to advance our understanding of the complex and promising world of few-body states in two-dimensional semiconductors.

Projects:

Trion Structure and Binding Energy Using Faddeev Method 

This project aims to develop a comprehensive theoretical framework and computational tools to study trions in semiconductor layered materials. The approach employs the Faddeev equations in momentum space, addressing the bound state of three distinct particles interacting with three different pair interactions in two dimensions. We utilize two different screening schemes for the repulsive electron-electron or hole-hole potential to solve the three coupled Faddeev integral equations for the Rytova-Keldysh interaction. One of these schemes screens the interaction in the infrared region, while the other screens it in the ultraviolet region. Our results demonstrate that both methods provide consistent outcomes for the MoS₂ layer, extrapolating the trion energy to the situation without screening. Specifically, we have found a trion binding energy of approximately -50 meV for an exciton energy of approximately −753 meV. Read more at arXiv.2212.09600.

Exciton Properties in Double-Layered TMDs

This project introduces a novel method for analyzing exciton properties in double-layered transition metal dichalcogenides (TMDs). Utilizing the Chebyshev polynomial expansion, we accurately solve the Wannier equation, integrating critical corrections for the quasiparticle bandgap. This approach allows for a systematic investigation of hetero double-layer TMD systems across a range of chemical compositions. The study primarily focuses on revealing how the spacer width and dielectric constant impact the binding energies of inter- and intralayer excitons. Read more at arXiv:2305.03576.

Four-Body Universality in 2D

The project aims to examine the universality of four-boson bound states in two dimensions. To achieve this, two different one-term separable potentials, featuring Gaussian and Yamaguchi form factors, are employed to calculate the ground and excited state energies of trimers and tetramers through the solution of Faddeev-Yakubovsky equations in momentum space. A key focus of the study is the exploration of the universality in the binding energies of tetramers and trimers and momentum distribution functions. This will be investigated across a broad spectrum of dimer binding energies and utilizing different form factor powers.

• K. Mohseni, M. R. Hadizadeh, T. Frederico, D. R. da Costa, A. J. Chaves, Trion clustering structure and binding energy in 2D semiconductor materials: Faddeev equations approach, Phys. Rev. B 107, 165427 (2023)
• Luiz G. M. Tenório, Teldo A. S. Pereira, K. Mohseni, T. Frederico, M. R. Hadizadeh, Diego R. da Costa, and André J. Chaves, Tunable properties of excitons in double monolayer semiconductor heterostructures, Phys. Rev. B 108, 035421 (2023)

• M. R. Hadizadeh, Bowling Green State University, Bowling Green, Ohio, March 20, 2024. Quantum Few-body Systems in Two Dimensions (seminar)
• M. R. Hadizadeh, K. Mohseni, A. J. Chaves, D. R. da Costa, T. Frederico, 2023 Fall Meeting of the APS-EGLS, Cleveland State University, Cleveland, Ohio, Oct. 21, 2023. Trions in Monolayer MoS2 using Faddeev Scheme in Momentum Space (talk)
• M. R. Hadizadeh, K. Mohseni, A. J. Chaves, D. R. da Costa, T. Frederico, NNCI Nano+Additive Manufacturing Summit, University of Louisville, Louisville, KY, July 26, 2023. A Numerical Solution of the Schrödinger Equation for Three-Charged Particle Bound Systems Utilizing the Faddeev Technique: A Detailed Analysis of Trions in a MoS2 Layer (talk)
• K. Mohseni, M. R. Hadizadeh, A. J. Chaves, D. R. da Costa, T. Frederico, The 2023 Autumn Meeting of the Brazilian Physical Society (EOSBF-2023), Ouro Preto - MG, Brazil, May 24, 2023. Trion structure in 2D materials: Faddeev equations approach (talk)
• M. R. Hadizadeh, K. Mohseni, T. Frederico, D. R. da Costa, A. J. Chaves, XVI International Conference on Nuclear Structure Properties (NSP2023), Karabük University, Karabük, Türkiye, May 9, 2023. Investigating few-body systems in 2D materials: adapting Faddeev method from nuclear physics (talk)
• M. R. Hadizadeh, K. Mohseni, A. J. Chaves, D. R. da Costa, T. Frederico, APS March Meeting, Las Vegas, Nevada, March 9, 2023. Application of the Faddeev technique to the bound states of three charged particles in two dimensions (talk)
• K. Mohseni, A. J. Chaves, D. R. da Costa, T. Frederico, M. R. Hadizadeh, 20th Brazilian Workshop On Semiconductor Physics, Aeronautics Institute of Technology (ITA), in São José dos Campos, São Paulo, Brazil, September 12, 2022. Few-body Physics in 2D materials (talk)
• Luiz G. M. Tenório, Teldo A S Pereira, K. Mohseni, T. Frederico, M. R. Hadizadeh, D. R. da Costa, and A. J. Chaves, 20th Brazilian Workshop On Semiconductor Physics, Aeronautics Institute of Technology (ITA), in São José dos Campos, São Paulo, Brazil, September 12, 2022. Tunable properties of excitons in double monolayer heterostructures (talk)
• K. Mohseni, A. J. Chaves, D. R. da Costa, T. Frederico, M. R. Hadizadeh, 20th Brazilian Workshop On Semiconductor Physics, Aeronautics Institute of Technology (ITA), in São José dos Campos, São Paulo, Brazil, September 12, 2022. Study negative trion structure in two dimensions using Faddeev equations approach (poster)

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Mohammadreza Hadizadeh

Associate Professor of Physics
CENS 264, Central State University
O: 937-376-6273
E: mhadizadeh@centralstate.edu
W: https://people.ohio.edu/hadizadm

• Andre J. Chaves, Adjunct Professor of Physics, Instituto Tecnológico de Aeronáutica, Brazil,
• Diego Rabelo da Costa, Adjunct Professor of Physics, Federal University of Ceará, Brazil,
• Tobias Frederico, Professor of Physics, Instituto Tecnológico de Aeronáutica, Brazil,
• Kamyar Mohseni, PhD candidate, Instituto Tecnológico de Aeronáutica, Brazil,
• Teldo A. S. Pereira, Adjunct Professor of Physics, Universidade Federal de Mato Grosso, Brazil,
• Luiz G. M. Tenório, PhD Student, RIKEN, Japan.